Don't Think So
There is no such command that I know of. If you wanted to make everything larger, you would need to edit all of the XML files yourself. Just so you understand, that would make just the windows larger. The game will still be rendered at 1024x768.
I wouldn't hold out hope that someone will make a larger UI. I think most of us feel the UI is oversized as it is. I have a feeling most of us are set on making it smaller, not larger.
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